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https://hdl.handle.net/20.500.14279/29828
Τίτλος: | Hydrogenation of carbon dioxide (CO2) to fuels in microreactors: a review of set-ups and value-added chemicals production | Συγγραφείς: | Hafeez, Sanaa Harkou, Eleana Al-Salem, Sultan M. Goula, Maria A. Dimitratos, Nikolaos Charisiou, Nikolaos D. Villa, Alberto Bansode, Atul Leeke, Gary Anthony Manos, George Constantinou, Achilleas |
Major Field of Science: | Medical and Health Sciences | Field Category: | Chemical Engineering | Λέξεις-κλειδιά: | Catalyst activity;Catalyst selectivity;Chemical reactors;Fossil fuels;Greenhouse effect;Hydrogenation;Industrial research;Solar power generation | Ημερομηνία Έκδοσης: | 10-Φεβ-2022 | Πηγή: | Reaction Chemistry and Engineering, 2022, vol. 7, iss. 4, pp. 795 - 812 | Volume: | 7 | Issue: | 4 | Start page: | 795 | End page: | 812 | Περίληψη: | Climate change, the greenhouse effect and fossil fuel extraction have gained a growing interest in research and industrial circles to provide alternative chemicals and fuel synthesis technologies. Carbon dioxide (CO2) hydrogenation to value-added chemicals using hydrogen (H2) from renewable power (solar, wind) offers a unique solution. From this aspect this review describes the various products, namely methane (C1), methanol, ethanol, dimethyl ether (DME) and hydrocarbons (HCs) originating via CO2 hydrogenation reaction. In addition, conventional reactor units for the CO2 hydrogenation process are explained, as well as different types of microreactors with key pathways to determine catalyst activity and selectivity of the value-added chemicals. Finally, limitations between conventional units and microreactors and future directions for CO2 hydrogenation are detailed and discussed. The benefits of such set-ups in providing platforms that could be utilized in the future for major scale-up and industrial operation are also emphasized. | URI: | https://hdl.handle.net/20.500.14279/29828 | DOI: | 10.1039/d1re00479d | Rights: | © Elsevier B.V. Attribution-NonCommercial-NoDerivatives 4.0 International |
Type: | Article | Affiliation: | University College London Cyprus University of Technology Kuwait Institute for Scientific Research University of Western Macedonia Università di Bologna Università degli Studi di Milano Delft University of Technology University of Birmingham |
Publication Type: | Peer Reviewed |
Εμφανίζεται στις συλλογές: | Άρθρα/Articles |
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