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Πεδίο DCΤιμήΓλώσσα
dc.contributor.authorSingh, Ranbir R.-
dc.contributor.authorPagona, Georgia-
dc.contributor.authorGregoriou, Vasilis G.-
dc.contributor.authorTagmatarchis, Nikos-
dc.contributor.authorToliopoulos, Dimosthenis-
dc.contributor.authorHan, Yang-
dc.contributor.authorFei, Zhuping-
dc.contributor.authorKatsouras, Athanasios-
dc.contributor.authorAvgeropoulos, Apostolos-
dc.contributor.authorAnthopoulos, Thomas D.-
dc.contributor.authorHeeney, Martin-
dc.contributor.authorKeivanidis, Panagiotis E.-
dc.contributor.authorChochos, Christos L.-
dc.date.accessioned2017-02-08T15:39:16Z-
dc.date.available2017-02-08T15:39:16Z-
dc.date.issued2015-04-28-
dc.identifier.citationPolymer Chemistry, 2015, vol. 6, iss. 16, pp. 3098-3109en_US
dc.identifier.issn17599962-
dc.identifier.urihttps://hdl.handle.net/20.500.14279/9542-
dc.description.abstractThe influence of the monomer's isomeric structure on the optical, electrochemical, charge transporting properties and photovoltaic performance of donor-acceptor (D-A) conjugated polymers has been demonstrated for the first time by studying two D-A copolymers consisting of bis(3-octyloxy)phenyl)quinoxaline as the electron deficient unit and the two isomeric structures of thienothiophene (thieno[3,2-b]thiophene and thieno[2,3-b]thiophene) as the electron rich units. The drastic effect of incorporating two different isomeric structures on the polymer backbone of these copolymers, manifests in changes observed in their optical, electrochemical and charge transporting properties. In contrast, the overall photovoltaic performance of the copolymers is similar, but distinct differences in the device photocurrents occur. These differences were attributed to morphology variations rather than the balanced mobility ratio. For further developments in the field, the isomeric structures of different functional monomers should be considered in the designing of new materials with even superior performance.en_US
dc.formatpdfen_US
dc.language.isoenen_US
dc.relation.ispartofPolymer Chemistryen_US
dc.rights© The Royal Society of Chemistryen_US
dc.subjectHeterojunction solar-cellsen_US
dc.subjectBand-gap copolymersen_US
dc.subjectConjugated polymersen_US
dc.subjectCharge-transporten_US
dc.subjectSemiconducting polymersen_US
dc.subjectOrganic electronicsen_US
dc.titleThe impact of thienothiophene isomeric structures on the optoelectronic properties and photovoltaic performance in quinoxaline based donor-acceptor copolymersen_US
dc.typeArticleen_US
dc.collaborationFondazione Istituto Italiano di Tecnologiaen_US
dc.collaborationAdvent Technologies SAen_US
dc.collaborationNational Hellenic Research Foundationen_US
dc.collaborationImperial College Londonen_US
dc.collaborationUniversity of Ioanninaen_US
dc.collaborationImperial College Londonen_US
dc.collaborationCyprus University of Technologyen_US
dc.subject.categoryChemical Sciencesen_US
dc.journalsSubscriptionen_US
dc.countryItalyen_US
dc.countryGreeceen_US
dc.countryUnited Kingdomen_US
dc.countryCyprusen_US
dc.subject.fieldNatural Sciencesen_US
dc.publicationPeer Revieweden_US
dc.identifier.doi10.1039/C5PY00075Ken_US
dc.relation.issue16en_US
dc.relation.volume6en_US
cut.common.academicyear2014-2015en_US
dc.identifier.spage3098en_US
dc.identifier.epage3109en_US
item.fulltextNo Fulltext-
item.languageiso639-1en-
item.grantfulltextnone-
item.openairecristypehttp://purl.org/coar/resource_type/c_6501-
item.cerifentitytypePublications-
item.openairetypearticle-
crisitem.journal.journalissn1759-9962-
crisitem.journal.publisherRoyal Society of Chemistry-
crisitem.author.deptDepartment of Mechanical Engineering and Materials Science and Engineering-
crisitem.author.deptDepartment of Mechanical Engineering and Materials Science and Engineering-
crisitem.author.facultyFaculty of Engineering and Technology-
crisitem.author.facultyFaculty of Engineering and Technology-
crisitem.author.orcid0000-0002-5336-249X-
crisitem.author.orcid0000-0002-7783-157X-
crisitem.author.parentorgFaculty of Engineering and Technology-
crisitem.author.parentorgFaculty of Engineering and Technology-
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