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https://hdl.handle.net/20.500.14279/9486
Πεδίο DC | Τιμή | Γλώσσα |
---|---|---|
dc.contributor.author | Ohta, Takehiro | - |
dc.contributor.author | Soulimane, Tewfik | - |
dc.contributor.author | Kitagawa, Teizo | - |
dc.contributor.author | Varotsis, Constantinos | - |
dc.date.accessioned | 2017-02-06T10:40:09Z | - |
dc.date.available | 2017-02-06T10:40:09Z | - |
dc.date.issued | 2015-04-28 | - |
dc.identifier.citation | Physical Chemistry Chemical Physics, 2015, vol. 17, no. 16, pp. 10894-10898. | en_US |
dc.identifier.issn | 14639076 | - |
dc.identifier.uri | https://hdl.handle.net/20.500.14279/9486 | - |
dc.description.abstract | Visible and UV-resonance Raman spectroscopy was employed to investigate the reaction of NO with cytochrome caa3 from Thermus thermophilus. We show the formation of the hyponitrite (HO–N[double bond, length as m-dash]N–O)− bound to the heme a3 species (νN[double bond, length as m-dash]N = 1330 cm−1) forming a high spin complex in the oxidized heme a3 Fe/CuB binuclear center of caa3-oxidoreductase. In the absence of heme a3 Fe2+–NO formation, the electron required for the formation of the N[double bond, length as m-dash]N bond originates from the autoreduction of CuB by NO, producing nitrite. With the identification of the hyponitrite intermediate the hypothesis of a common phylogeny of aerobic respiration and bacterial denitrification is fully supported and the mechanism for the 2e−/2H+ reduction of NO to N2O can be described with more certainty. | en_US |
dc.format | en_US | |
dc.language.iso | en | en_US |
dc.relation.ispartof | Physical Chemistry Chemical Physics | en_US |
dc.rights | © The Owner Societies | en_US |
dc.rights | Attribution-NonCommercial-NoDerivs 3.0 United States | * |
dc.rights.uri | http://creativecommons.org/licenses/by-nc-nd/3.0/us/ | * |
dc.subject | Nitric oxide | en_US |
dc.subject | Thermus thermophilus | en_US |
dc.title | Nitric oxide activation by caa3 oxidoreductase from Thermus thermophilus | en_US |
dc.type | Article | en_US |
dc.collaboration | University of Hyogo | en_US |
dc.collaboration | University of Limerick | en_US |
dc.collaboration | Cyprus University of Technology | en_US |
dc.subject.category | Chemical Sciences | en_US |
dc.journals | Subscription | en_US |
dc.country | Japan | en_US |
dc.country | Ireland | en_US |
dc.country | Cyprus | en_US |
dc.subject.field | Natural Sciences | en_US |
dc.publication | Peer Reviewed | en_US |
dc.identifier.doi | 10.1039/c5cp01013f | en_US |
dc.relation.issue | 16 | en_US |
dc.relation.volume | 17 | en_US |
cut.common.academicyear | 2015-2016 | en_US |
dc.identifier.spage | 10894 | en_US |
dc.identifier.epage | 108 | en_US |
item.fulltext | No Fulltext | - |
item.languageiso639-1 | en | - |
item.grantfulltext | none | - |
item.openairecristype | http://purl.org/coar/resource_type/c_6501 | - |
item.cerifentitytype | Publications | - |
item.openairetype | article | - |
crisitem.journal.journalissn | 1463-9084 | - |
crisitem.journal.publisher | Royal Society of Chemistry | - |
crisitem.author.dept | Department of Chemical Engineering | - |
crisitem.author.faculty | Faculty of Geotechnical Sciences and Environmental Management | - |
crisitem.author.orcid | 0000-0003-2771-8891 | - |
crisitem.author.parentorg | Faculty of Geotechnical Sciences and Environmental Management | - |
Εμφανίζεται στις συλλογές: | Άρθρα/Articles |
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